Computergames... the ./hack and the the various Final Fantasy OSTs are worth listening to, although the FF ones are Import only as I recall so they'll be pricey to buy.
Anime Soundtracks? Akira for sure! Also Hellsing (it's very different from most other Anime OSTs, but this is no bad thing at all).
Wolf's Rain , Voices of a Distant Star, Grave of the Fireflies, and Someday's Dreamers are personal favourites. dkstranger suggested Haibane Renmei, Last Exile, Witch Hunter Robin, or anything by Yoko Kannoor Yuki Kajiura. He aslo says Miyazaki and studio Ghibli have good soundracks.
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But I reccomend Silent hill 2-3 as well as anything by Squaresoft...
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Anime Soundtracks? Akira for sure! Also Hellsing (it's very different from most other Anime OSTs, but this is no bad thing at all).
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http://gh.ffshrine.org/
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But thanks- it's a bloody brilliant site!